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The effect of an HP-beta-CD-functionalized metal-organic framework on lanthanide cations.
The stepwise inclusion of lanthanide ions by a dicarboxylate complex, 2,3-naphthoquinonediazido (NQD), into a metal-organic framework, comprising a 3,5-connected network of Ti(4)O(2)(OH)(2) vertices, was investigated using a combination of infrared spectroscopy, ion chromatography, nuclear magnetic resonance spectroscopy, solid-state (57)Cu NMR, and X-ray absorption spectroscopy. Evidence for all steps of the inclusion process was obtained. The presence of HP-beta-CD, 2-adamantanemethanoic acid, 4-hydroxybenzoic acid, as well as 1-benzyl-3-methylimidazole-2-thione (BMIT) was required for the detection of either a 16-membered ring (Ln(NQD)(2)) or a 14-membered ring (Ln(NQD)(2)). The matrix selectivity of the dic
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